Highly selective CO2 removal for one-step liquefied natural gas processing by physisorbents
Author | Madden, David G. |
Author | O'Nolan, Daniel |
Author | Chen, Kai Jie |
Author | Hua, Carol |
Author | Kumar, Amrit |
Author | Pham, Tony |
Author | Forrest, Katherine A. |
Author | Space, Brian |
Author | Perry, John J. |
Author | Khraisheh, Majeda |
Author | Zaworotko, Michael J. |
Available date | 2020-08-18T08:34:43Z |
Publication Date | 2019 |
Publication Name | Chemical Communications |
Resource | Scopus |
ISSN | 13597345 |
Abstract | Industrial specifications require CO2 concentrations in natural gas below 50 ppm during liquefaction because of corrosion and CO2 freezing. Herein, we report a physisorbent (TIFSIX-3-Ni) that exhibits new benchmark CO2/CH4 selectivity and fast kinetics, thereby enabling one-step LNG processing to CO2 levels of 25 ppm. - 2019 The Royal Society of Chemistry. |
Sponsor | M. J. Z. acknowledges SFI (13/RP/B2549 and 16/IA/4624). M. J. Z. and M. K. acknowledge QNRF (NPRP10-0107-170119). T. P., K. A. F., and B. S. acknowledges the National Science Foundation (Award No. DMR-1607989), including support from the Major Research Instrumentation Program (Award No. CHE-1531590). Computational resources were made available by a XSEDE Grant (No. TG-DMR090028) and by Research Computing at the University of South Florida. T. P. and B. S. also acknowledges support from a ACS Petroleum Research Fund grant (ACS PRF 56673-ND6). |
Language | en |
Publisher | Royal Society of Chemistry |
Subject | Metal-Organic Frameworks Schl�fli Symbol Isophthalate |
Type | Article |
Pagination | 3219-3222 |
Issue Number | 22 |
Volume Number | 55 |
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