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المؤلفLu, Qingqing
المؤلفEid, Kamel
المؤلفLi, Wenpeng
المؤلفAbdullah, Aboubakr M.
المؤلفXu, Guobao
المؤلفVarma, Rajender S.
تاريخ الإتاحة2022-09-26T06:08:48Z
تاريخ النشر2021-08-07
اسم المنشورGreen Chemistry
المعرّفhttp://dx.doi.org/10.1039/d1gc01303c
الاقتباسLu, Q., Eid, K., Li, W., Abdullah, A. M., Xu, G., & Varma, R. S. (2021). Engineering graphitic carbon nitride (gC 3 N 4) for catalytic reduction of CO 2 to fuels and chemicals: strategy and mechanism. Green Chemistry, 23(15), 5394-5428.‏
الرقم المعياري الدولي للكتاب14639262
معرّف المصادر الموحدhttps://www.scopus.com/inward/record.uri?partnerID=HzOxMe3b&scp=85112353264&origin=inward
معرّف المصادر الموحدhttp://hdl.handle.net/10576/34443
الملخصThe reduction of carbon dioxide to useful fuels/chemicals, such as methane, formic, and methanol, is an innovative way to address looming energy and environmental issues. Graphitic carbon nitride (g-C3N4), as a greener and low-cost catalyst for the electrocatalytic and photocatalytic carbon dioxide reduction reaction (CO2RR) to provide usable fuels, is endowed with numerous appealing attributes, e.g., Earth-abundant resources, facile synthesis, metal-free nature, catalytic properties, and unique thermal-physical-chemical stability. Articles on the use of g-C3N4 for CO2 transformation have increased significantly in the past decade, and it is important to provide timely updates in this emerging and active research area. This review emphasizes the rational structural engineering of g-C3N4, including doping (i.e., metal, non-metal, and molecular) and heterojunction formation (i.e., metal, metal oxide, metal phosphide, metal hydroxide, metal complex, Ag-halides, and carbon materials) for electrocatalytic, photoelectrocatalytic, and photocatalytic CO2RR. Besides, an in-depth deciphering of the CO2RR mechanism from experimental, theoretical, and fundamental concepts is provided, including deliberation on the sources/emission and strategies to avoid/reduce CO2 emission. Lastly, a brief conclusion and outlook on the challenges and future prospects are highlighted to assist further in the rational design of the g-C3N4-based catalyst as a selective and efficient catalyst for the CO2RR.
اللغةen
الناشرRoyal Society of Chemistry
الموضوعcarbon nitride
العنوانEngineering graphitic carbon nitride (g-C3N4) for catalytic reduction of CO2 to fuels and chemicals: strategy and mechanism
النوعArticle Review
الصفحات5394-5428
رقم العدد15
رقم المجلد23
dc.accessType Abstract Only


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