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    CO 2 adsorption studies on Prussian blue analogues

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    Date
    2012
    Author
    Karadas, F.
    El-Faki, H.
    Deniz, E.
    Yavuz, C.T.
    Aparicio, S.
    Atilhan, M.
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    Abstract
    Carbon dioxide (CO2) adsorption capacities of several Prussian blue (PB) analogues have been studied using the state-of-the-art Rubotherm® sorption apparatus to obtain adsorption and desorption isotherms of these compounds up to 50 bar. The analogues were prepared by simply reacting a [M(CN)6]3− (Mdouble bondCo, Fe) solution with solutions of M2+ (Mdouble bondMn, Fe, Co, Ni, Cu) metal ions. Characterization of the studied samples has been performed by using a combination of powder XRD, TGA, FTIR, and CHN elemental analysis. Adsorption capacities of PB analogues calculated with theoretical calculations, using Monte Carlo approach, have also been compared with the experimental study, and used to discuss the molecular mechanism of adsorption.
    DOI/handle
    http://dx.doi.org/10.1016/j.micromeso.2012.06.019
    http://hdl.handle.net/10576/40287
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    • Chemical Engineering [‎1194‎ items ]

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